长江口及邻近海域表层沉积物中重金属元素含量分布及其影响因素

董爱国; 翟世奎; ZABELMatthias; 于增慧

长江口及邻近海域表层沉积物中重金属元素含量分布及其影响因素

1.
中国海洋大学, 海底科学与探测技术教育部重点实验室, 山东, 青岛, 266100;不来梅大学, 海洋地球科学学院, 不来梅, D-28334
2.
中国海洋大学, 海底科学与探测技术教育部重点实验室, 山东, 青岛, 266100
3.
不来梅大学, 海洋地球科学学院, 不来梅, D-28334

基金项目: 国家重大基础研究规划“九七三”项目资助(2002CB412409)

计量
- 文章访问数: 1299
- HTML全文浏览量: 9
- PDF下载量: 1288
- 被引次数: 0
出版历程
- 收稿日期: 2008-04-16
- 修回日期: 2009-03-06

The distribution of heavy metal contents in surface sediments of the Changjiang Estuary in China and surrounding coastal areas

1.
Key Laboratory of Submarine Geosciences and Prospecting Techniques of Ministry of Education, Ocean University of China, Qingdao 266100, China;Fachbereich Geowissenschaften, Universität Bremen, Postfach 330440, D-28334, Germany
2.
Key Laboratory of Submarine Geosciences and Prospecting Techniques of Ministry of Education, Ocean University of China, Qingdao 266100, China
3.
Fachbereich Geowissenschaften, Universität Bremen, Postfach 330440, D-28334, Germany

摘要

摘要: 根据2003和2006年长江口及邻近海域表层沉积物样品的粒度组成和元素铬、铜、镍、铅、锌、铝、钙和锶的含量,分析了重金属元素含量的分布特征,探讨了含量的变化趋势及其对人类活动的响应。自2003年三峡工程一期蓄水完成到2006年6月,长江输沙量逐年减少,长江口海域沉积物中黏土的百分含量明显增加,但是沉积物分布的总体格局并没有发生明显的变化。重金属元素大多在泥质区沉积物中富集,高值区沿岸线呈带状分布,在最大浑浊带和口外羽状锋处达到峰值。在长江大量物质输入的背景下,研究区沉积物中重金属元素含量相对其他类似河口较低。河流的陆源颗粒输入、水动力条件、细颗粒物质的吸附以及絮凝作用是控制沉积物中重金属元素含量分布的主要因素,氧化还原条件也对重金属元素含量变化有一定的影响。人类活动(重大工程的建设和人为污染)对长江口外泥质区中重金属元素含量有重要影响,尤其对铅和锌的含量及其分布的影响显著。自2003年三峡工程一期蓄水以来,长江口海域表层沉积物中重金属元素沉积机制未有明显的变化,但是重金属元素含量有逐渐降低的趋势。
- 长江口海域 /
- 表层沉积物 /
- 重金属元素 /
- 三峡工程一期蓄水
Abstract: In order to discuss the response of heavy metals to human activities, two cruises'data in 2003and 2006 and surface sediments were collected in the Changjiang Estuary and its surrounding coastal areas. Contents of some elements (chromium, copper, nickel, lead, zinc, calcium and strontium) and grainsize composition were analyzed. The result showed that there were no significant changes in the pattern of sediment distribution, although the percentages of clay component increased significantly. The low content and zone-type distribution of heavy metals were observed and heavy metals were enriched in an mud area. And the two areas of heavy metal high contents were located in the turbidity maximum zone and the west of plume front which was caused by the mixing between diluted water and seawater. Terrigenous discharge, hydrographic dynamics, adsorption and flocculation played important role in the distribution of heavy metals. In addition, the redox condition and the human activity which was more important for lead and zinc, were also two important factors. The Phase-Ⅰ engineering of Sanxia Reservoir stored water since 2003, there had been not obvious change in the heavy metal deposition mechanism of surface sediments in the Changjiang Estuary, but the contents of heavy metals had a gradually decreasing trend.
- Changjiang Estuary in China /
- surface sediment /
- heavy metal element /
- Sanxia Reservoir

HTML全文

参考文献(32)

金翔龙.东海海洋地质[M].北京:海洋出版社,1992:524.

秦蕴珊,赵一阳,陈丽蓉,等.东海地质[M].北京:科学出版社,1987:290.

MILLIMAN D John,SHEN Huang-ting,YANG Zuo-sheng,et al.Transport and deposition of river sediment in the Changjiang Estuary and adjacent continental shelf[J].Continental Shelf Research,1985,4:37-45.

赵一阳.中国海大陆架沉积物地球化学的若干模式[J].地质科学,1983,4:307-313.

赵一阳,焉明才.中国浅海沉积物地球化学[M].北京:科学出版社,1994:203.

孟翊,刘苍宇.长江口区沉积地球化学特征的定量研究[J].华东师范大学学报(自然科学版),1996,1:73-84.

LIN Saulwood,HSIEH I-Jy,HUANG Kuo-ming,et al.Influence of the Yangtze River and grain size of the spatial variation of heavy metals and organic carbon in the East China Sea continental shelf sediment[J].Chemical Geology,2002,182:377-394.

CHEN Zhong-yuan,SAITO Y,KANAI Y,et al.Low concentration of heavy metals in the Yangtze estuarine sediments,Chinas a diluting setting[J].Estuarine,Coastal and Shelf Science,2004,60s 91-100.

中华人民共和国水利部.中国河流泥沙公报[R].北京:中国水利水电出版社,2006.

肖尚斌,李安春,蒋富清,等.近2 ka闽浙沿岸泥质沉积物物源分析[J].沉积学报,2005,23(2):268-274.

李双林,李绍全,孟祥君.东海陆架晚第四纪沉积物化学成分及物源示踪[J].海洋地质与第四纪地质,2002,22(4):21-28.

苏纪兰,袁业立.中国近海水文[M].北京:海洋出版社,2005:367.

郭志刚,杨作升,曲艳慧,等.东海陆架泥质区沉积地球化学比较研究[J].沉积学报,2000,18(2):284-289.

许淑梅,张晓东,翟世奎,等.长江口及其邻近海域表层沉积物粒度划分及变化规律研究[J].海洋地质动态,2007,23(2):1-8.

SAITO Y,YANG Zuo-sheng.Historical change of the Huanghe (Yellow River) and its impact on the sediment budget of the East China Sea[C]//TSUNOGAI S,ISEKI K,KOIKE I,et al.Proceedings of international symposium on the global fluxes of carbon and its related substances in the coastal ocean atmosphere system.Sapporo,Japans Hokkido University,1994:7-12.

李道季,张经,黄大吉,等.长江口外氧的亏损[J].中国科学(D辑),2002,32(8):686-694.

海洋图集编委会.渤海黄海东海海洋图集:水文分册[Q].北京:海洋出版社,1992.524.

ZABEL M,SCHNEIDER R R,WAGNER T,et al.Late quaternary climate changes in central Africa as inferred from terrigenous input to the Niger Fan[J].Quaternary Research,2001,56:207-217.

张怀静,翟世奎,范德江,等.三峡工程一期蓄水后长江口及其邻近海域悬浮物浓度分布特征[J].环境科学,2007,28(8):1655-1661.

ZOU Huai-yang,PENG Xiao-tong,PAN Jing-ming.Distribution,source and enrichment of some chemical elements in sediments of the Pearl River Estuary,China[J].Continental Shelf Research,2004,24:1857-1875.

ZHANG Jing,HUANG Wei-wen,MARTIN J M.Trace metals distribution in Huanghe (Yellow River) estuarine sediments[J].Estuarine,Coastal and Shelf Science,1988,26:499-516.

ATTRI M J,THOMAS R.Heavy metal concentrations in sediment from the Thames estuary,UK[J].Marine Pollution Bulletin,1995,34 (10):742-744.

TUREDIAN K K,WEDEPOHL K H.Distribution of the elements in some major units of the earth's crust[J].Bulletin of the Geological Society of America,1961,72,175-192.

魏复盛,陈静生,吴燕玉,等.中国土壤环境背景值研究[J].环境科学,1991,12(4):12-19.

TAYLOR S R.Abundance of chemical elements in the continental crust:a new table[J].Geochimica et Cosmochimica Acta,1964,28:1273-1285.

齐红艳,范德江,徐琳.等.长江口及邻近海域表层沉积物pH,Eh分布及制约因素[J].沉积学报,2008,26(5);820-827.

沈焕庭,潘定安.长江河口最大浑浊带[M].北京:海洋出版社,2001:194.

张怀静,翟世奎,范德江,等.三峡工程一期蓄水后长江口悬浮体形态及物质组成[J].海洋地质与第四纪地质,2007,27(2):1-10.

夏福兴,陈敏,陈邦林.长江口最大浑浊带悬浮颗粒中有机重金属的异常[J].华东师范大学学报,1996,1:52-56.

KOSCHINSKY A.Heavy metal distributions in Peru Basin surface sediments in relation to historic,present and disturbed redox environments[J].Deep-Sea Research (Ⅱ),2001,48:3757-3777.

IP C M C,LI Xiang-dong,ZHANG Gan,et al.Trace metal distribution in sediments of the Pearl River Estuary and the surrounding coastal area,South China[J].Environmental Pollution,2007,147:311-323.

BIRTH G.A scheme for assessing human impacts on coastal aquatic environments using sediments[C]//WOODCOFFE C D,FURNESS R A.Coastal GIS.Australia:Wollongong University Papers in Center for Maritime Policy,2003:14.

施引文献

资源附件(0)

访问统计